Crowne Plaza is definitely located in the best district (Gare de Lyon is mainly a soulless business district) :
located in the Haut Marais, full of trendy boutiques and restaurants (by the way, I am suprised that the hotel has not been transformed into a Kimpton hotel, as the area is definitely fits more with the positioning than Opéra, where only tourists go).
Some good spots at walkable distance from the hotel (less than 10 minutes walk) :
Season organic restaurant
Broken arm, trendy boutique
Anahi, great Argentine restaurant
Hôtel Providence, with very good restaurant (with some French stars)
Copper Bay, excellent cocktail bar
Chiche, warm and friendly Israelian restaurant
House of 3 brothers, excellent contemporary patisserie
Yann couvreur, another great pâtissier
Chateaubriand, excellent bistronomique restaurant
Candaleria, one of the coolest bar in Paris
Popelini, so chou!
PNY burger, tasty and design
Galerie Chantal Crousel, one of the most avant garde art galleries in Paris
Merci, creative concept store with a café
Maison Plisson, food to buy or to eat at restaurant
Maison Kitsuné, one of the most trendy French fashion label (with a café)
Renaissance République, with a hidden, quiet and very pleasant garden (restaurant and bar)
All the districts North (Canal Saint Martin), North East (Ménilmontant) and South of the hotel (Marais) are one of the most trendy areas in Paris.
Enjoy!